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Acid-leached alpha-MnO2 nanowires for electrochemical energy storage
Conference proceeding

Acid-leached alpha-MnO2 nanowires for electrochemical energy storage

Bryan Byles, Arunkumar Subramanian and Ekaterina Pomerantseva
NANOEPITAXY: MATERIALS AND DEVICES VI, v 9174, pp 91740Z-91740Z-8
01 Jan 2014

Abstract

Engineering Engineering, Electrical & Electronic Materials Science Materials Science, Multidisciplinary Optics Physical Sciences Physics Physics, Applied Science & Technology Technology
We present synthesis, acid-leaching, characterization and electrochemistry of alpha-MnO2 nanowires with tunnel crystal structure. This material is used as a matrix for lithium ions intercalation to provide insights into the effects of postsynthesis treatment on charge storage properties. Hydrothermal treatment of precursors produced 20 - 200 nm thick and tens of microns long nanowires. Acid leaching was carried out in the concentrated nitric acid at room temperature and resulted in the change of material composition and surface area. Original alpha-MnO2 nanowires showed initial discharge specific capacity of 96 mAh/g, while acid-leached material exhibited higher capacity values. This work forms the basis for future study aimed at understanding of correlation between crystal structure, composition and morphology of the "host" matrix and nature of the "guest" ions for beyond lithium electrochemical energy storage. In addition, we demonstrate single nanowire electrochemical cells for the study of electrochemically-correlated mechanical properties of the nanowires.

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Collaboration types
Domestic collaboration
Web of Science research areas
Engineering, Electrical & Electronic
Materials Science, Multidisciplinary
Optics
Physics, Applied
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