Logo image
A MEMS platform for in situ, real-time monitoring of electrochemically induced mechanical changes in lithium-ion battery electrodes
Journal article   Peer reviewed

A MEMS platform for in situ, real-time monitoring of electrochemically induced mechanical changes in lithium-ion battery electrodes

Ekaterina Pomerantseva, Hyun Jung, Markus Gnerlich, Sergio Baron, Konstantinos Gerasopoulos, Reza Ghodssi and Energy Frontier Research Centers (EFRC)
Journal of micromechanics and microengineering, v 23(11), pp 114018/1-114018/10
01 Nov 2013

Abstract

electrode Fabry-Perot interferometer lithium-ion battery thin film volume expansion contraction
We report the first successful demonstration of an optical microelectromechanical systems (MEMS) sensing platform for the in situ characterization of electrochemically induced reversible mechanical changes in lithium-ion battery (LIB) electrodes. The platform consists of an array of flexible membranes with a reflective surface on one side and a thin-film LIB electrode on the other side. The membranes deflect due to the active battery material volume change caused by lithium intercalation (expansion) and extraction (contraction). This deflection is monitored using the Fabry-Perot optical interferometry principle. The active material volume change causes high internal stresses and mechanical degradation of the electrodes. The stress evolution observed in a silicon thin-film electrode incorporated into this MEMS platform follows a 'first elastic, then plastic' deformation scheme. Understanding of the internal stresses in battery electrodes during discharge charge is important for improving the reliability and cycle lifetime of LIBs. The developed MEMS platform presents a new method for in situ diagnostics of thin-film LIB electrodes to aid the development of new materials, optimization of electrode performance, and prevention of battery failure.

Metrics

4 Record Views
10 citations in Scopus

Details

UN Sustainable Development Goals (SDGs)

This publication has contributed to the advancement of the following goals:

#11 Sustainable Cities and Communities

InCites Highlights

Data related to this publication, from InCites Benchmarking & Analytics tool:

Web of Science research areas
Engineering, Electrical & Electronic
Instruments & Instrumentation
Nanoscience & Nanotechnology
Physics, Applied
Logo image