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Amplification-by-Polymerization in Biosensing for Human Genomic DNA Detection
Journal article   Peer reviewed

Amplification-by-Polymerization in Biosensing for Human Genomic DNA Detection

Peng He, Xinhui Lou, Susan M Woody and Lin He
ACS sensors, v 4(4), pp 992-1000
26 Apr 2019
PMID: 30942069

Abstract

biosensors amplification-by-polymerization RAFT genomic DNA detection ATRP
A polymerization reaction was employed as a signal amplification method to realize direct visualization of gender-specific DNA extracted from human blood in a polymerase chain reaction (PCR)-free fashion. Clear distinction between X and Y chromosomes was observed by naked eyes for detector-free sensing purposes. The grown polymer films atop X and Y chromosomes were quantitatively measured by ellipsometry for thickness readings. Detection assays have been optimized for genomic DNA recognition to a maximum extent by varying the selection of the proper blocking reagents, the annealing temperature, and the annealing time. Traditional PCR and gel electrophoresis for amplicon identification were conducted in parallel for performance comparison. In the blind test for blood samples examined by the new approach, 25 out of 26 were correct and one was false negative, which was comparable to, if not better than, the PCR results. This is the first time our amplification-by-polymerization technique is being used for chromosome DNA analysis. The potential of adopting the described sensing technique without PCR was demonstrated, which could further promote the development of a portable, PCR-free DNA sensing device for point-of-need applications.

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Collaboration types
Domestic collaboration
International collaboration
Web of Science research areas
Chemistry, Analytical
Chemistry, Multidisciplinary
Nanoscience & Nanotechnology
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