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Biomimetic proteoglycans diffuse throughout articular cartilage and localize within the pericellular matrix
Journal article   Peer reviewed

Biomimetic proteoglycans diffuse throughout articular cartilage and localize within the pericellular matrix

Evan R. Phillips, Brett D. Haislup, Nicholas Bertha, Maria Lefchak, Joseph Sincavage, Katsiaryna Prudnikova, Brandon Shallop, Mary K. Mulcahey and Michele S. Marcolongo
Journal of biomedical materials research. Part A, v 107(9), pp 1977-1987
01 Sep 2019
PMID: 31056821

Abstract

Engineering Engineering, Biomedical Materials Science Materials Science, Biomaterials Science & Technology Technology
Biomimetic proteoglycan (BPG) diffusion into articular cartilage has the potential to restore the lost proteoglycan content in osteoarthritic cartilage given these molecules mimic the structure and properties of natural proteoglycans. We examined the diffusion characteristics of BPGs through cartilage with the use of a custom-made in vitro cartilage diffusion model in both normal bovine and human osteoarthritic cartilage explants. BPGs were introduced into the cartilage through essentially one-dimensional diffusion using osteochondral plugs. The molecular diffusion was shown to be size and concentration dependent. Diffusion profiles were found over different diffusion time intervals and the profiles were fit to a nonlinear Fickian diffusion model. Steady state 011012-7diffusion coefficients for BPGs were found to be 4.01 and 3.53 mu m(2)/s for 180 and 1600 kDa BPGs, respectfully, and these values are similar to other large molecule diffusion in cartilage. In both bovine and osteoarthritic human cartilage, BPGs were found localized around the chondrocytes. BPG localization was examined by labeling collagen type VI and soaking 5 mu m thick sections of cartilage with BPG solutions demonstrating that the BPGs diffused into the cartilage and preferentially localized alongside collagen type VI in the pericellular matrix.

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14 citations in Scopus

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Collaboration types
Domestic collaboration
Web of Science research areas
Engineering, Biomedical
Materials Science, Biomaterials
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