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Electron beam modification and functionalization of MWNT for covalent dispersion into polymeric systems
Journal article

Electron beam modification and functionalization of MWNT for covalent dispersion into polymeric systems

Mary E. Sullivan, Don Klosterman and Giuseppe R. Palmese
Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, v 265(1), pp 352-355
01 Dec 2007

Abstract

Instruments & Instrumentation Nuclear Science & Technology Physical Sciences Physics Physics, Atomic, Molecular & Chemical Physics, Nuclear Science & Technology Technology
The development of nanotube-based polymer composites with improved mechanical properties and electrical conductivity requires the covalent dispersion of carbon nanotubes to utilize their stress transfer capabilities. Covalent dispersion of nanotubes therefore requires the functionalization of their surface to interact with solvents or monomers. In this work, we have developed a novel method of nanotube surface modification in which dry MANT are irradiated with a high-energy electron beam (EB) in ambient air environment. Raman spectroscopy was performed to characterize the influence of EB irradiation on nanotubes, namely, variance of the disorder, or D band (similar to 1360 cm(-1)) with respect to the graphitic, or G, band (similar to 1580 cm(-1)). Raman spectra show increased deformation to the graphitic structure, as well as increased strain on the carbon-carbon bonds, weakening the nanotube. Transmission electron microscopy (TEM) confirms that nanotubes remain intact despite high EB dose. In addition, minimal surface deformation and length reduction occurred on irradiated MWNT. (c) 2007 Elsevier B.V. All rights reserved.

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Collaboration types
Domestic collaboration
Web of Science research areas
Instruments & Instrumentation
Nuclear Science & Technology
Physics, Atomic, Molecular & Chemical
Physics, Nuclear
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