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Emission and transmission Mossbauer spectroscopic (EMS and TMS) study of perovskite oxides, (Ba, Ca)(Fe, Co)O3-delta absorbed with CO2
Journal article   Peer reviewed

Emission and transmission Mossbauer spectroscopic (EMS and TMS) study of perovskite oxides, (Ba, Ca)(Fe, Co)O3-delta absorbed with CO2

K Nomura, Z Homonnay, G Vanko, A Vertes, L Poppl, A Nath, Y Ujihira, T Hayakawa and K Takehira
Hyperfine interactions, v 112(1-4), pp 7-12
01 Jan 1998

Abstract

Physical Sciences Physics Physics, Atomic, Molecular & Chemical Physics, Condensed Matter Physics, Nuclear Science & Technology
Perovskite oxides, (Ba0.95Ca0.05) (Co1-x,Fe-x) O3-delta, are prominent materials for CO, absorption at high temperature. The substitution of Ba sites with Ca ion, and the mixed valence states of Fe and Co ions due to the formation of oxygen vacancies at high temperatures are effective for CO2 absorption. Especially Co ions are more active for CO absorption than Fe ions. These oxides were analyzed by EMS and TMS before and after treatment in CO2 atmospheres. The difference between EMS and TMS spectra is found to be observed not only due to the oxygen affinity, but also to the different reactivity of Co and Fe ions in the B site towards CO2.

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Collaboration types
Domestic collaboration
International collaboration
Web of Science research areas
Physics, Atomic, Molecular & Chemical
Physics, Condensed Matter
Physics, Nuclear
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