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Fracture Characterization of Recycled High Density Polyethylene/Nanoclay Composites Using the Essential Work of Fracture Concept
Journal article   Open access   Peer reviewed

Fracture Characterization of Recycled High Density Polyethylene/Nanoclay Composites Using the Essential Work of Fracture Concept

Sukjoon Na, Sabrina Spatari and Yick G. Hsuan
Polymer engineering and science, v 56(2)
01 Feb 2016
DOI: https://doi.org/10.1002/pen.24250
Featured in Collection :   UN Sustainable Development Goals @ Drexel
url
https://doi.org/10.1002/pen.24250View
Published, Version of Record (VoR)Maybe Open Access (Publisher Bronze),  Open

Abstract

Engineering Engineering, Chemical Physical Sciences Polymer Science Science & Technology Technology
The effect of nanoclay on the plane-strain fracture behavior of pristine High density polyethylene (HDPE) and recycled HDPE blends was studied using the essential work of fracture (EWF) concept. The failure mode of EWF tested specimens was found to be associated with the specific non-EWF (beta(B)w(p,B)). Adding 6-wt% of nanoclay to pristine HDPE and 2-wt% to recycle-blends greatly decreased the beta(B)w(p,B) values and led to a transition from ductile to brittle failure mode. A fractographic study revealed that the difference in failure modes was caused by the changes in micro and macro morphologies, which could be related with the specific EWF (w(e,B)). In the ductile failure, w(e,B) is governed by the fibril size; adding nanoclay and recycled HDPE to pristine HDPE decreased the fibril size and subsequently lowered the w(e,B) value. In the brittle failure, the w(e,B) value was enhanced by creating a rough fracture surface. Adding nanoclay to pristine HDPE, a steadily decrease in w(e,B) was measured until 4-wt% after which the change was insignificant. Conversely, nanoclay content more than 2-wt% in recycle-blends greatly decreased the w(e,B) value. A transition map was constructed to illustrate the potential failure mode and the associated fracture morphology based on the tested material compositions. (C) 2015 Society of Plastics Engineers

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6 citations in Web of Science
9 citations in Scopus

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Web of Science research areas
Engineering, Chemical
Polymer Science
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