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Fructose Accelerates UV-C Induced Photochemical Degradation of Pentachlorophenol in Low and High Salinity Water
Journal article   Peer reviewed

Fructose Accelerates UV-C Induced Photochemical Degradation of Pentachlorophenol in Low and High Salinity Water

Shaila Nayak, Sean-Erik O'Donnell, Christopher M. Sales and Rohan V. Tikekar
Journal of agricultural and food chemistry, v 64(21), pp 4214-4219
01 Jun 2016
PMID: 27160945

Abstract

Agriculture, Multidisciplinary Chemistry Chemistry, Applied Food Science & Technology Life Sciences & Biomedicine Science & Technology Agriculture Physical Sciences
A novel process involving 254 nm UV-C and fructose to degrade pentachlorophenol (PCP), a pollutant, in low and high salinity (0-10 g/L salt) solutions is presented. The first order rate constants in the presence of 0, 300, and 500 mM fructose were 0.23 +/- 0.04, 0.54 +/- 0.01, and 1.18 +/- 0.03 min(-1), respectively. Experimental evidence has shown generation of hydrogen peroxide and singlet oxygen from the UV-C exposure of fructose, which may have accelerated PCP degradation. Although salts (sodium, potassium, and calcium chloride, 1101:6.4:1) are expected to enhance the degradation rate due to generation of reactive halide species (RHS) from exposure to UV-C light, 10 g/L salt decreased the degradation rates in both the absence and presence of fructose. An LC-ESI-MS spectrum of the reaction mixture revealed a high relative abundance at m/z of 215 that corresponds to a fructose-chlorine adduct, indicating that fructose may have scavenged these RHS and prevented their reaction with PCP.

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UN Sustainable Development Goals (SDGs)

This publication has contributed to the advancement of the following goals:

#6 Clean Water and Sanitation

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Collaboration types
Domestic collaboration
Web of Science research areas
Agriculture, Multidisciplinary
Chemistry, Applied
Food Science & Technology
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