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Mechanistic Investigation of the Inhibition of Aβ42 Assembly and Neurotoxicity by Aβ42 C-terminal Fragments
Journal article   Open access   Peer reviewed

Mechanistic Investigation of the Inhibition of Aβ42 Assembly and Neurotoxicity by Aβ42 C-terminal Fragments

Huiyuan Li, Bernhard H Monien, Aleksey Lomakin, Reeve Zemel, Erica A Fradinger, Miao Tan, Sean M Spring, Brigita Urbanc, Cui-Wei Xie, George B Benedek, …
Biochemistry (Easton), v 49(30), pp 6358-6364
03 Aug 2010
PMID: 20568734
url
https://doi.org/10.1021/bi100773gView
Published, Version of Record (VoR) Open

Abstract

dynamic light scattering aggregation neurotoxicity inhibitor Amyloid β-protein
Oligomeric forms of amyloid β-protein (Aβ) are key neurotoxins in Alzheimer's disease (AD). Previously, we found that C-terminal fragments (CTFs) of Aβ42 interfered with assembly of full-length Aβ42 and inhibited Aβ42-induced toxicity. To decipher the mechanism(s) by which CTFs affect Aβ42 assembly and neurotoxicity, here, we investigated the interaction between Aβ42 and CTFs using photo-induced cross-linking and dynamic light scattering. The results demonstrate that distinct parameters control CTF inhibition of Aβ42 assembly and Aβ42-induced toxicity. Inhibition of Aβ42-induced toxicity was found to correlate with stabilization of oligomers with hydrodynamic radius ( R H ) = 8–12 nm and attenuation of formation of oligomers with R H = 20–60 nm. In contrast, inhibition of Aβ42 paranucleus formation correlated with CTF solubility and the degree to which CTFs formed amyloid fibrils themselves but did not correlate with inhibition of Aβ42-induced toxicity. Our findings provide an important insight into the mechanisms by which different CTFs inhibit the toxic effect of Aβ42 and suggest that stabilization of non-toxic Aβ42 oligomers is a promising strategy for designing inhibitors of Aβ42 neurotoxicity.

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Collaboration types
Domestic collaboration
Web of Science research areas
Biochemistry & Molecular Biology
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