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Metallic Ti 3 C 2 T x MXene Gas Sensors with Ultrahigh Signal-to-Noise Ratio
Journal article   Open access   Peer reviewed

Metallic Ti 3 C 2 T x MXene Gas Sensors with Ultrahigh Signal-to-Noise Ratio

Seon Joon Kim, Hyeong-Jun Koh, Chang E Ren, Ohmin Kwon, Kathleen Maleski, Soo-Yeon Cho, Babak Anasori, Choong-Ki Kim, Yang-Kyu Choi, Jihan Kim, …
ACS nano, v 12(2), pp 986-993
27 Feb 2018
PMID: 29368519
url
https://doi.org/10.1021/acsnano.7b07460View
Published, Version of Record (VoR)Open Access (Publisher-Specific) Open

Abstract

gas sensing MXene metallic channel signal-to-noise ratio titanium carbide two-dimensional materials volatile organic compound ESI Highly Cited Paper (Incites)
Achieving high sensitivity in solid-state gas sensors can allow the precise detection of chemical agents. In particular, detection of volatile organic compounds (VOCs) at the parts per billion (ppb) level is critical for the early diagnosis of diseases. To obtain high sensitivity, two requirements need to be simultaneously satisfied: (i) low electrical noise and (ii) strong signal, which existing sensor materials cannot meet. Here, we demonstrate that 2D metal carbide MXenes, which possess high metallic conductivity for low noise and a fully functionalized surface for a strong signal, greatly outperform the sensitivity of conventional semiconductor channel materials. Ti C T MXene gas sensors exhibited a very low limit of detection of 50-100 ppb for VOC gases at room temperature. Also, the extremely low noise led to a signal-to-noise ratio 2 orders of magnitude higher than that of other 2D materials, surpassing the best sensors known. Our results provide insight in utilizing highly functionalized metallic sensing channels for developing highly sensitive sensors.

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Collaboration types
Domestic collaboration
International collaboration
Web of Science research areas
Chemistry, Multidisciplinary
Chemistry, Physical
Materials Science, Multidisciplinary
Nanoscience & Nanotechnology
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