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Migration of Aluminum Atoms in the Transformation of γ–to θ–Alumina
Journal article

Migration of Aluminum Atoms in the Transformation of γ–to θ–Alumina

Shu-Hui Cai and Karl Sohlberg
MRS proceedings, v 731
2002

Abstract

γ– and θ–alumina are two metastable phases of aluminum oxide observed along the thermal dehydration sequence of boehmite before conversion to the final product α–alumina. The transformation from γ– to θ–alumina was studied by using Al16O24 cells. Motion of some Al atoms from their γalumina positions to new positions and no O motions result in an approximate structure that, upon relaxation by first-principles calculations, becomes the known θ–alumina structure. Total-energy calculations along the paths of the atomic motions have been used to map out transformation pathways. The model accurately predicts experimentally observed domain boundaries in θ–alumina and the γ– to θ–alumina conversion rate.

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Web of Science research areas
Materials Science, Characterization & Testing
Mathematics, Applied
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