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Journal article
MoS 2 -on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries
Angewandte Chemie (International ed.), v 57(7), pp 1846-1850
12 Feb 2018
PMID: 29292844
Featured in Collection : UN Sustainable Development Goals @ Drexel
Abstract
Two-dimensional (2D) heterostructured materials, combining the collective advantages of individual building blocks and synergistic properties, have spurred great interest as a new paradigm in materials science. The family of 2D transition-metal carbides and nitrides, MXenes, has emerged as an attractive platform to construct functional materials with enhanced performance for diverse applications. Here, we synthesized 2D MoS
-on-MXene heterostructures through in situ sulfidation of Mo
TiC
T
MXene. The computational results show that MoS
-on-MXene heterostructures have metallic properties. Moreover, the presence of MXene leads to enhanced Li and Li
S adsorption during the intercalation and conversion reactions. These characteristics render the as-prepared MoS
-on-MXene heterostructures stable Li-ion storage performance. This work paves the way to use MXene to construct 2D heterostructures for energy storage applications.
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Details
- Title
- MoS 2 -on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries
- Creators
- Chi Chen - School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, P. R. ChinaXiuqiang Xie - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USABabak Anasori - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USAAsya Sarycheva - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USATaron Makaryan - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USAMengqiang Zhao - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USAPatrick Urbankowski - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USALing Miao - School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, P. R. ChinaJianjun Jiang - School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, P. R. ChinaYury Gogotsi - A.J. Drexel Nanomaterials Institute, Materials Science and Engineering Department, Drexel University, 3141 Chestnut Street, Philadelphia, PA, 19104, USA
- Publication Details
- Angewandte Chemie (International ed.), v 57(7), pp 1846-1850
- Publisher
- Wiley; Germany
- Resource Type
- Journal article
- Language
- English
- Academic Unit
- Materials Science and Engineering
- Web of Science ID
- WOS:000424212300015
- Scopus ID
- 2-s2.0-85040713408
- Other Identifier
- 991014969861304721
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- Collaboration types
- Domestic collaboration
- International collaboration
- Web of Science research areas
- Chemistry, Multidisciplinary