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Monitoring oxidation of multiwalled carbon nanotubes by Raman spectroscopy
Journal article   Open access   Peer reviewed

Monitoring oxidation of multiwalled carbon nanotubes by Raman spectroscopy

Sebastian Osswald, Mickael Havel and Yury Gogotsi
Journal of Raman spectroscopy, v 38(6), pp 728-736
Jun 2007
url
https://doi.org/10.1002/jrs.1686View
Published, Version of Record (VoR)Maybe Open Access (Publisher Bronze) Open

Abstract

functionalization oxidation nanotube
Multiwalled carbon nanotubes (MWCNTs) were oxidized in air and acids while varying the treatment time and/or temperature. The goal of this approach was to create the highest density of carboxyl groups with moderate sample loss, which is necessary for nanocomposite applications. In situ Raman experiments allowed real‐time observation of the structural changes in MWCNTs upon oxidation. The ratio of the Raman intensities of the D and G bands was used to estimate the concentration of defects. It was found that while an oxidation for 6 h in H2SO4/HNO3 provided the strongest effect, a ‘flash oxidation’ in air (15 min at 550 °C) also leads to an efficient functionalization in a cost‐effective and environmentally friendly way. Transmission electron microscopy, Fourier‐transform infrared (FTIR) spectroscopy, thermogravimetric analysis and electrophoretic mobility analysis were used to study the oxidized nanotubes. Copyright © 2007 John Wiley & Sons, Ltd.

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