Order-to-disorder transition due to entropy in layered and 2D carbides

This work was supported by the National Science Foundation (Center for Chemical Innovation M-STAR program grant CHE-2318105 to B.C.W., Y.Y., T.P., Y.M., F.U., G.K., M.T., S.K.N., A.B., H.F., K.K., B.G.W., R.D., A.T., S.H., Z.F., Y.G., A.V., D.J., and B.A.; Solid State & Materials Chemistry program grant DMR-2419026 to B.C.W., S.K.N., A.B., K.K., B.G.W., R.D., A.T., and B.A.; grant CBET-2051525 to J.J., N.G., and X.X.); National Science Centre, Poland (SONATA BIS 142024/54/E/ST11/00171 to P.P.M.); National Centre for Research and Development, Poland (LIDER XII LIDER/8/0055/L-12/20/NCBR/2021 to P.P.M.); Laboratory Directed Research and Development (LDRD) of Argonne National Laboratory, Office of Science, US Department of Energy (contract DE-AC02-06CH11357 to S.P.M. and Z.D.H.); the Vagelos Institute for Energy Science and Technology, University of Pennsylvania (graduate fellowship to Y.M.); the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility (supported by the Office of Science of the US Department of Energy contract DE-AC02-05CH11231 using NERSC award BES-ERCAP0023161 to Y.M. and A.V.); and the Ministry of Trade, Industry, and Energy (MOTIE) Korea (Global Industrial Technology Cooperation Center program grant P0028332 supervised by the Korea Institute for Advancement of Technology to B.C.W., Y.G., and B.A.).