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Some nickel(II) complexes with pentadentate and tridentate heterocyclic N- and S-donor ligands
Journal article   Peer reviewed

Some nickel(II) complexes with pentadentate and tridentate heterocyclic N- and S-donor ligands

Jayakumar G Gilbert, Anthony W Addison and Raymond J Butcher
Inorganica Chimica Acta, v 308(1), pp 22-30
2000

Abstract

Crystal structures N- and S-donor complexes Nickel complexes Polydentate ligand complexes
High-spin Ni(II) complexes of the linear pentadentate ligand 2,6-bis([2′-aminophenylthio]methyl)pyridine (Batp) and the tridentate ligands ([2′-aminophenylthio]ethyl)pyridine (Atep) 1,5-bis( N-methylbenzimidazol-2′-yl)-3-oxapentane (Mbeo) have been prepared. Crystal structures of the complexes [Ni(Batp)(H 2O)](CF 3SO 3) 2 ( 2) and [Ni(Atep) 2](ClO 4) 2 ( 4) reveal pseudooctahedral coordination. Tetragonal distortion in [Ni(Mbeo) 2](ClO 4) 2 ( 5) is evident from the longer Ni–O and shorter Ni–N bond lengths. From the electronic spectrum of 5, the tetragonal distortion parameter D t and the in-plane Dq xy and axial Dq z ligand field parameters are calculated. The three Ni(II) complexes exhibit irreversible cathodic electrochemistry.

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Collaboration types
Domestic collaboration
Web of Science research areas
Chemistry, Inorganic & Nuclear
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