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Synthesis, Structure, and Spectroscopy of Epitaxial EuFeO3 Thin Films
Journal article   Peer reviewed

Synthesis, Structure, and Spectroscopy of Epitaxial EuFeO3 Thin Films

Amber K. Choquette, Robert Colby, Eun Ju Moon, Christian M. Schlepuetz, Mark D. Scafetta, David J. Keavney, Steven J. May and Pacific Northwest National Laboratory (PNNL), Richland, WA (US), Environmental Molecular Sciences Laboratory (EMSL)
Crystal growth & design, v 15(3), pp 1105-1111
01 Mar 2015

Abstract

Chemistry Chemistry, Multidisciplinary Crystallography Materials Science Materials Science, Multidisciplinary Physical Sciences Science & Technology Technology
Rare earth iron perovskites RFeO3, where R is a rare earth cation, exhibit an array of magnetic, catalytic, optical, and electrochemical properties. Here we study EuFeO3 films synthesized by molecular beam epitaxy to improve our understanding of the optical properties of ferrites. A combination of X-ray diffraction, X-ray reflectivity, Rutherford backscattering spectroscopy, and scanning transmission electron microscopy was used to characterize the film structure and cation composition. X-ray absorption spectroscopy confirms the nominal 3+ valence states of Eu and Fe. The optical properties of EuFeO3 were investigated using variable-angle spectroscopic ellipsometry between the photon energies of 1.25 and 5 eV. We find that EuFeO3 is a semiconductor with an onset of optical absorption near 2.5 eV. The absorption spectrum of EuFeO3 is blue-shifted with respect to LaFeO3 films, a result that is attributed to the structural differences between the two materials.

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Collaboration types
Domestic collaboration
Web of Science research areas
Chemistry, Multidisciplinary
Crystallography
Materials Science, Multidisciplinary
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