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Synthesis and characterization of electroactive and biodegradable ABA block copolymer of polylactide and aniline pentamer
Journal article   Peer reviewed

Synthesis and characterization of electroactive and biodegradable ABA block copolymer of polylactide and aniline pentamer

Lihong Huang, Jun Hu, Le Lang, Xin Wang, Peibiao Zhang, Xiabin Jing, Xianhong Wang, Xuesi Chen, Peter I. Lelkes, Alan G. MacDiarmid, …
Biomaterials, v 28(10), pp 1741-1751
2007
PMID: 17218007

Abstract

Aniline pentamer Biocompatibility Biodegradable Electroactive Polylactide
A triblock copolymer PLA- b-AP- b-PLA (PAP) of polylactide (PLA) and aniline pentamer (AP) with the unique properties of being both electroactive and biodegradable is synthesized by coupling an electroactive carboxyl-capped AP with two biodegradable bi-hydroxyl-capped PLAs via a condensation reaction. Three different molecule weight PAP copolymers are prepared. The PAP copolymers exhibit excellent electroactivity similar to the AP and polyaniline, which may stimulate cell proliferation and differentiation. The electrical conductivity of the PAP2 copolymer film (∼5×10 −6 S/cm) is in the semiconducting region. Transmission electron microscopic results suggest that there is microphase separation of the two block segments in the copolymer, which might contribute to the observed conductivity. The biodegradation and biocompatibility experiments in vitro prove the copolymer is biodegradable and biocompatible. Moreover, these new block copolymer shows good solubility in common organic solvents, leading to the system with excellent processibility. These biodegradable PAP copolymers with electroactive function thus possess the properties that would be potentially used as scaffold materials for neuronal or cardiovascular tissue engineering.

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Domestic collaboration
International collaboration
Web of Science research areas
Engineering, Biomedical
Materials Science, Biomaterials
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