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The importance of experimental design on measurement of dynamic interfacial tension and interfacial rheology in diffusion-limited surfactant systems
Journal article   Open access   Peer reviewed

The importance of experimental design on measurement of dynamic interfacial tension and interfacial rheology in diffusion-limited surfactant systems

Matthew D. Reichert, Nicolas J. Alvarez, Carlton F. Brooks, Anne M. Grillet, Lisa A. Mondy, Shelley L. Anna and Lynn M. Walker
Colloids and surfaces. A, Physicochemical and engineering aspects, v 467, pp 135-142
20 Feb 2015
url
https://doi.org/10.1016/j.colsurfa.2014.11.035View
Accepted (AM)Open Access (Publisher-Specific) Open

Abstract

CiEj Interfacial elasticity Nonionic surfactant Pendant bubble Pendant drop
•Guidelines for design of interfacial rheology measurements that incorporate curvature and surfactant isotherm.•Interfacial mechanics using a pendant drop/bubble.•Scaling to design dynamic interfacial tension experiments on curved interfaces.•Demonstration of scaling using experiments and simulations. Pendant bubble and drop devices are invaluable tools in understanding surfactant behavior at fluid–fluid interfaces. The simple instrumentation and analysis are used widely to determine adsorption isotherms, transport parameters, and interfacial rheology. However, much of the analysis performed is developed for planar interfaces. The application of a planar analysis to drops and bubbles (curved interfaces) can lead to erroneous and unphysical results. We revisit this analysis for a well-studied surfactant system at air–water interfaces over a wide range of curvatures as applied to both expansion/contraction experiments and interfacial elasticity measurements. The impact of curvature and transport on measured properties is quantified and compared to other scaling relationships in the literature. The results provide tools to design interfacial experiments for accurate determination of isotherm, transport and elastic properties.

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Collaboration types
Domestic collaboration
Web of Science research areas
Chemistry, Physical
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