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iCVD growth of poly(N-vinylimidazole) and poly (N-vinylimidazole-co-N-vinylpyrrolidone)
Journal article   Peer reviewed

iCVD growth of poly(N-vinylimidazole) and poly (N-vinylimidazole-co-N-vinylpyrrolidone)

Guohua Chen, Kenneth K. S. Lau and Karen K. Gleason
Thin solid films, v 517(12), pp 3539-3542
30 Apr 2009

Abstract

Materials Science Materials Science, Coatings & Films Materials Science, Multidisciplinary Physical Sciences Physics Physics, Applied Physics, Condensed Matter Science & Technology Technology
The imidazole group plays an important role in alpha-chymotrypsin catalysis, metal-ion complexation, counterion or dye binding. Poly(N-vinylimidazole), PVI, is also a good model polymer interacting with neutral salts. The poly(N-vinylimidazole-co-N-vinylpyrrolidone) copolymer P(VI-co-VP), can be used to produce highly functionalized polymers. PVI and P(VI-co-VP) thins films were achieved via initiated chemical vapor deposition (iCVD), a solvent-free process to form films under mild conditions. The polymerization was initiated by hot wire heated tert-butyl peroxide (TBPO). The chemical structure and compositions of the polymers were analyzed using FTIR and XPS. The growth rate of PVI as a function of the pressure inside the iCVD reactor was measured to be 1 nm/h mTorr. The XPS results show that the functional groups were retained in the polymer deposited. For the P(VI-co-VP) deposition, there are more VI groups found in the co-polymer chain even when the reacting monomers were fed in the same ratio. (C) 2009 Elsevier B.V. All rights reserved.

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Web of Science research areas
Materials Science, Coatings & Films
Materials Science, Multidisciplinary
Physics, Applied
Physics, Condensed Matter
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