Journal article
High-resolution extrusion printing of Ti3C2-based inks for wearable human motion monitoring and electromagnetic interference shielding
Carbon (New York), v 191, pp 277-289
May 2022
Abstract
This work addresses two major challenges of MXene-based printing; that is, its low printing resolution (i.e., filament spreading >120%) and its inability to create structures with simultaneously high electrical conductivity and mechanical flexibility. We first report high-resolution extrusion printing of Ti3C2 and composite of Ti3C2/poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS). The printing has a negligible filament spreading (<25%) and low thickness and width variations (<20%) compared to their average values. We then fabricate Ti3C2/PEDOT:PSS composite structures that possess simultaneously exceptional electrical conductivity and flexibility (conductivity of 1600 ± 400 S/cm for 80 wt% Ti3C2, which can withstand up to 3000 bending cycles). Addressing the two challenges expands the applications of MXene-based printing. For instance, micrometer-thick grids printed with our method show excellent EMI shielding effectiveness and superior specific EMI shielding effectiveness, reaching 38.4 dB and 43,000 dB cm2 g−1 in the case of pure Ti3C2 and 28.1 dB and 32,000 dB cm2 g−1 for the composite containing 80 wt% Ti3C2. The printed structures of pure Ti3C2 also perform as highly-sensitive strain sensors with a gauge factor of 11,300 at a strain of 4%. The prepared sensors are capable of monitoring various human activities, including breathing, facial muscles movements, and talking.
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•Aqueous and additive-free inks of pure Ti3C2 and composites Ti3C2/PEDOT:PSS were developed.•High-resolution extrusion printing of Ti3C2-based inks was demonstrated.•Printed structures of Ti3C2 showed simultaneously high conductivity and mechanical flexibility.•Printed grids of Ti3C2-based inks showed unique EMI shielding characteristics.•Printed structures of pure Ti3C2 were performed as highly-sensitive strain sensors.
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Details
- Title
- High-resolution extrusion printing of Ti3C2-based inks for wearable human motion monitoring and electromagnetic interference shielding
- Creators
- Ahmadreza Ghaffarkhah - MBIAMilad Kamkar - MBIAZahra Azimi Dijvejin - University of TorontoHossein Riazi - Drexel UniversitySaeed Ghaderi - MBIAKevin Golovin - University of TorontoMasoud Soroush - Drexel UniversityMohammad Arjmand - MBIA
- Publication Details
- Carbon (New York), v 191, pp 277-289
- Publisher
- Elsevier
- Resource Type
- Journal article
- Language
- English
- Academic Unit
- Chemical and Biological Engineering
- Web of Science ID
- WOS:000760412400006
- Scopus ID
- 2-s2.0-85124186010
- Other Identifier
- 991019169645404721
InCites Highlights
Data related to this publication, from InCites Benchmarking & Analytics tool:
- Collaboration types
- Domestic collaboration
- International collaboration
- Web of Science research areas
- Chemistry, Physical
- Materials Science, Multidisciplinary